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This option also worked well for me (Tarik) in Jan-14. I just waited for 15 minutes until a gracious Spanish couple gave me a ride to Girona.
This option worked for me (Joel) too in June-15. Waited 20 minutes before I was picked up by some really friendly spaniards. The trouble for me was to get out of Spain (gave up after 4 hours) and I was stuck just close to the border to France in La Jonquera before I finally had to get a cab to Perpignan. Apparently -nobody- picks up hitch hikers just next to the border because this is a huge drug smuggling zone. Both 2 rides I took before they clearly asked me if I had any drugs on me. I had no idea why but now I understand. My recommendation is that you find someone that goes all the way to France in Montcada / Girona, because believe me, there is absolutely nothing to see in La Jonquera. (In hindsight I should've just walked the remaining 5 kms to France where it's very easy to catch a ride.)
==== Option 2: Bellaterra ====